A complete quantum description of an ultrafast pump-probe charge transfer event in condensed phase

The development of methodological tools for modeling ultrafast dynamics in a dissipative environment was studied. The Hamiltonian method was found to suit the ultrafast events because it was not limited by weak coupling between environment and system. This method was applied to a pump probe experimental description, where each step of the cycle was consistently treated. The nonadiabatic dynamics was found to be sensitive to all internal system parameters and system-bath coupling elements.