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A shorter 146Sm half-life measured and implications for 146Sm-142Nd chronology in the solar system

  • N. Kinoshita
  • , M. Paul*
  • , Y. Kashiv
  • , P. Collon
  • , C. M. Deibel
  • , B. DiGiovine
  • , J. P. Greene
  • , D. J. Henderson
  • , C. L. Jiang
  • , S. T. Marley
  • , T. Nakanishi
  • , R. C. Pardo
  • , K. E. Rehm
  • , D. Robertson
  • , R. Scott
  • , C. Schmitt
  • , X. D. Tang
  • , R. Vondrasek
  • , A. Yokoyama
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

162 Scopus citations

Abstract

The extinct p-process nuclide 146Sm serves as an astrophysical and geochemical chronometer through measurements of isotopic anomalies of its α-decay daughter 142Nd. Based on analyses of 146Sm/147Sm α-activity and atom ratios, we determined the half-life of 146Sm to be 68 ± 7 (1σ) million years, which is shorter than the currently used value of 103 ± 5 million years. This half-life value implies a higher initial 146Sm abundance in the early solar system, (146Sm/144Sm)0 = 0.0094 ± 0.0005 (2σ), than previously estimated. Terrestrial, lunar, and martian planetary silicate mantle differentiation events dated with 146Sm-142Nd converge to a shorter time span and in general to earlier times, due to the combined effect of the new 146Sm half-life and (146Sm/144Sm)0 values.

Original languageEnglish
Pages (from-to)1614-1617
Number of pages4
JournalScience
Volume335
Issue number6076
DOIs
StatePublished - 30 Mar 2012

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