Atom-phonon interactions studied using a consistent quantum treatment

Charles Cerjan*, Ronnie Kosloff

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

20 Scopus citations

Abstract

A consistent approach to atomsurface-energy transfer in one dimension is presented. A semigroup technique is employed to establish equations of motion for a quantal phonon reservoir, which is coupled to the propagation of a wave packet. The time-dependent Schrödinger equation is solved using a pseudospectral technique. The average energy transfer to the bath is then determined. This study supersedes conventional perturbative treatments and reveals the utility of one-dimensional models in the study of particle-surface collisions at low energies.

Original languageEnglish
Pages (from-to)3832-3840
Number of pages9
JournalPhysical Review B
Volume34
Issue number6
DOIs
StatePublished - 1986

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