Coarse-grained lattice models for drying-mediated self-assembly of nanoparticles

Orly Kletenik-Edelman; Claudia G. Sztrum-Vartash; Eran Rabani

doi:10.1039/b817439c

Coarse-grained lattice models for drying-mediated self-assembly of nanoparticles

Orly Kletenik-Edelman^*
, Claudia G. Sztrum-Vartash
, Eran Rabani

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

22 Scopus citations

Abstract

We present a coarse-grained lattice gas approach applicable for modelling the drying-mediated self-assembly of nanoparticles. The approach is exemplified for self-assembly of binary superlattices and for the hierarchical self-assembly of nanoparticles over patterned templates. The theory predicts many observed superstructures along with novel morphologies yet to be explored. The role of solvent evaporation, nanoparticle diffusion mechanisms, surface patterning, and the relevant time and length scales are discussed.

Original language	English
Pages (from-to)	2872-2876
Number of pages	5
Journal	Journal of Materials Chemistry
Volume	19
Issue number	19
DOIs	https://doi.org/10.1039/b817439c
State	Published - 2009
Externally published	Yes

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abstract = "We present a coarse-grained lattice gas approach applicable for modelling the drying-mediated self-assembly of nanoparticles. The approach is exemplified for self-assembly of binary superlattices and for the hierarchical self-assembly of nanoparticles over patterned templates. The theory predicts many observed superstructures along with novel morphologies yet to be explored. The role of solvent evaporation, nanoparticle diffusion mechanisms, surface patterning, and the relevant time and length scales are discussed.",

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AB - We present a coarse-grained lattice gas approach applicable for modelling the drying-mediated self-assembly of nanoparticles. The approach is exemplified for self-assembly of binary superlattices and for the hierarchical self-assembly of nanoparticles over patterned templates. The theory predicts many observed superstructures along with novel morphologies yet to be explored. The role of solvent evaporation, nanoparticle diffusion mechanisms, surface patterning, and the relevant time and length scales are discussed.

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Coarse-grained lattice models for drying-mediated self-assembly of nanoparticles

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