Coherent vibrational spectroscopy of barrier descent dynamics

M. Ben-Nun; R. D. Levine

doi:10.1016/0009-2614(93)85291-U

Coherent vibrational spectroscopy of barrier descent dynamics

M. Ben-Nun^*, R. D. Levine

^*Corresponding author for this work

Institute of Chemistry

Research output: Contribution to journal › Article › peer-review

11 Scopus citations

Abstract

Coherent product vibrational motion is demonstrated in computational studies of barrier dynamics for both gas phase and liquid phase processes. The coherence decays primarily due to intramolecular anharmonicity. Caging by the liquid tends to reduce the initial dephasing. Real time, short pulse, electronic spectroscopy can discern the vibrational coherence.

Original language	English
Pages (from-to)	450-456
Number of pages	7
Journal	Chemical Physics Letters
Volume	203
Issue number	5-6
DOIs	https://doi.org/10.1016/0009-2614(93)85291-U
State	Published - 5 Mar 1993

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title = "Coherent vibrational spectroscopy of barrier descent dynamics",

abstract = "Coherent product vibrational motion is demonstrated in computational studies of barrier dynamics for both gas phase and liquid phase processes. The coherence decays primarily due to intramolecular anharmonicity. Caging by the liquid tends to reduce the initial dephasing. Real time, short pulse, electronic spectroscopy can discern the vibrational coherence.",

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AB - Coherent product vibrational motion is demonstrated in computational studies of barrier dynamics for both gas phase and liquid phase processes. The coherence decays primarily due to intramolecular anharmonicity. Caging by the liquid tends to reduce the initial dephasing. Real time, short pulse, electronic spectroscopy can discern the vibrational coherence.

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Coherent vibrational spectroscopy of barrier descent dynamics

Abstract

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