TY - JOUR
T1 - Coupled-Trajectory Quantum-Classical Approach to Electronic Decoherence in Nonadiabatic Processes
AU - Min, Seung Kyu
AU - Agostini, Federica
AU - Gross, E. K.U.
N1 - Publisher Copyright:
© 2015 American Physical Society.
PY - 2015/8/10
Y1 - 2015/8/10
N2 - We present a novel quantum-classical approach to nonadiabatic dynamics, deduced from the coupled electronic and nuclear equations in the framework of the exact factorization of the electron-nuclear wave function. The method is based on the quasiclassical interpretation of the nuclear wave function, whose phase is related to the classical momentum and whose density is represented in terms of classical trajectories. In this approximation, electronic decoherence is naturally induced as an effect of the coupling to the nuclei and correctly reproduces the expected quantum behavior. Moreover, the splitting of the nuclear wave packet is captured as a consequence of the correct approximation of the time-dependent potential of the theory. This new approach offers a clear improvement over Ehrenfest-like dynamics. The theoretical derivation presented in this Letter is supported by numerical results that are compared to quantum mechanical calculations.
AB - We present a novel quantum-classical approach to nonadiabatic dynamics, deduced from the coupled electronic and nuclear equations in the framework of the exact factorization of the electron-nuclear wave function. The method is based on the quasiclassical interpretation of the nuclear wave function, whose phase is related to the classical momentum and whose density is represented in terms of classical trajectories. In this approximation, electronic decoherence is naturally induced as an effect of the coupling to the nuclei and correctly reproduces the expected quantum behavior. Moreover, the splitting of the nuclear wave packet is captured as a consequence of the correct approximation of the time-dependent potential of the theory. This new approach offers a clear improvement over Ehrenfest-like dynamics. The theoretical derivation presented in this Letter is supported by numerical results that are compared to quantum mechanical calculations.
UR - http://www.scopus.com/inward/record.url?scp=84939486214&partnerID=8YFLogxK
U2 - 10.1103/PhysRevLett.115.073001
DO - 10.1103/PhysRevLett.115.073001
M3 - ???researchoutput.researchoutputtypes.contributiontojournal.article???
AN - SCOPUS:84939486214
SN - 0031-9007
VL - 115
JO - Physical Review Letters
JF - Physical Review Letters
IS - 7
M1 - 073001
ER -