TY - JOUR
T1 - Dielectric maximum temperature non-monotonic behavior in unaxial Sr 0.75Ba0.25Nb2O6 relaxor seen via acoustic emission
AU - Dul-kin, E.
AU - Kojima, S.
AU - Roth, M.
PY - 2011/8/15
Y1 - 2011/8/15
N2 - [100] oriented Sr0.75Ba0.25Nb2O 6 relaxor crystals have been studied by means of acoustic emission (AE) over a wide 20-400° C temperature range. Both the Burns temperature, Td = 350° C, and the intermediate temperature, T* = 183°C, and the susceptibility maximum temperature, Tm (59° C on heating and 47° C on cooling), have been successfully detected. Dependent upon the external electric field, the Tm exhibits a local minimum near 0.25 kV=cm accompanied by pronounced AE maximum in a manner which had recently been detected in Pb(Mg1/3Nb2/3)O3-0.33PbTiO 3 by Dul-kin et al. [Appl. Phys. Lett. 94, 252904 (2009)] and in Pb(Sc1/2Ta1/2)O3 by Dul-kin et al. [Phys. Rev. B 82, 180101(R) (2010)], whereas the T* increases monotonically, similar to that which had recently been revealed in BaTiO3 by Dul-kin et al. [Appl. Phys. Lett. 97, 032903 (2010)] with a rate of 7.5 K cm/kV. An observed Tm behavior is discussed from the point of view of the existence of the random electric field components along the [100] direction in Sr0.75Ba0.25Nb2O6 crystals.
AB - [100] oriented Sr0.75Ba0.25Nb2O 6 relaxor crystals have been studied by means of acoustic emission (AE) over a wide 20-400° C temperature range. Both the Burns temperature, Td = 350° C, and the intermediate temperature, T* = 183°C, and the susceptibility maximum temperature, Tm (59° C on heating and 47° C on cooling), have been successfully detected. Dependent upon the external electric field, the Tm exhibits a local minimum near 0.25 kV=cm accompanied by pronounced AE maximum in a manner which had recently been detected in Pb(Mg1/3Nb2/3)O3-0.33PbTiO 3 by Dul-kin et al. [Appl. Phys. Lett. 94, 252904 (2009)] and in Pb(Sc1/2Ta1/2)O3 by Dul-kin et al. [Phys. Rev. B 82, 180101(R) (2010)], whereas the T* increases monotonically, similar to that which had recently been revealed in BaTiO3 by Dul-kin et al. [Appl. Phys. Lett. 97, 032903 (2010)] with a rate of 7.5 K cm/kV. An observed Tm behavior is discussed from the point of view of the existence of the random electric field components along the [100] direction in Sr0.75Ba0.25Nb2O6 crystals.
UR - http://www.scopus.com/inward/record.url?scp=80052413976&partnerID=8YFLogxK
U2 - 10.1063/1.3622670
DO - 10.1063/1.3622670
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AN - SCOPUS:80052413976
SN - 0021-8979
VL - 110
JO - Journal of Applied Physics
JF - Journal of Applied Physics
IS - 4
M1 - 044106
ER -