Abstract
We report on the direct observation of stretched exponential relaxation in low-temperature monatomic Lennard-Jones systems which were cooled slowly from the liquid phase to form crystals with a large number of defects. We use the cage correlation function [E. Rabani, J. D. Gezelter, and B. J. Berne, J. Chem. Phys. 107, 6867 (1997)] which measures changes in atomic surroundings to observe the stretched exponential relaxations. We obtain a distribution of hopping rates assuming that the origin of the Kohlrausch-Williams-Watts law is from static disorder in the distribution of barrier heights.
| Original language | English |
|---|---|
| Pages (from-to) | 3649-3652 |
| Number of pages | 4 |
| Journal | Physical Review Letters |
| Volume | 82 |
| Issue number | 18 |
| DOIs | |
| State | Published - 1999 |
| Externally published | Yes |
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