Even-harmonic generation due to beyond-born-oppenheimer dynamics

Thomas Kreibich, Volker Engel, E. K. Gross, Manfred Lein

Research output: Contribution to journalArticlepeer-review

8 Scopus citations

Abstract

Nonadiabatic effects in an oriented and isotopically asymmetric diatomic molecule lead to the emission of even harmonics. Such effects are particularly intense at high-harmonic frequencies. This information is relevant not only from a fundamental point of view, but also has the practical implication that reliable spectra can be obtained from fixed-nuclei calculations.

Original languageAmerican English
Article number103901
Pages (from-to)103901/1-103901/4
JournalPhysical Review Letters
Volume87
Issue number10
StatePublished - 3 Sep 2001
Externally publishedYes

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