High-Mobility, Wet-Transferred Graphene Grown by Chemical Vapor Deposition

  • Domenico De Fazio
  • , David G. Purdie
  • , Anna K. Ott
  • , Philipp Braeuninger-Weimer
  • , Timofiy Khodkov
  • , Stijn Goossens
  • , Takashi Taniguchi
  • , Kenji Watanabe
  • , Patrizia Livreri
  • , Frank H.L. Koppens
  • , Stephan Hofmann
  • , Ilya Goykhman
  • , Andrea C. Ferrari
  • , Antonio Lombardo*
  • *Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

161 Scopus citations

Abstract

We report high room-temperature mobility in single-layer graphene grown by chemical vapor deposition (CVD) after wet transfer on SiO2 and hexagonal boron nitride (hBN) encapsulation. By removing contaminations, trapped at the interfaces between single-crystal graphene and hBN, we achieve mobilities up to ∼70000 cm2 V-1 s-1 at room temperature and ∼120...000 cm2 V-1 s-1 at 9K. These are more than twice those of previous wet-transferred graphene and comparable to samples prepared by dry transfer. We also investigate the combined approach of thermal annealing and encapsulation in polycrystalline graphene, achieving room-temperature mobilities of ∼30...000 cm2 V-1 s-1. These results show that, with appropriate encapsulation and cleaning, room-temperature mobilities well above 10...000 cm2 V-1 s-1 can be obtained in samples grown by CVD and transferred using a conventional, easily scalable PMMA-based wet approach.

Original languageEnglish
Pages (from-to)8926-8935
Number of pages10
JournalACS Nano
Volume13
Issue number8
DOIs
StatePublished - 27 Aug 2019
Externally publishedYes

Bibliographical note

Publisher Copyright:
Copyright © 2019 American Chemical Society.

Keywords

  • CVD
  • charge carrier mobility
  • graphene
  • heterostructures
  • transfer

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