Intensity effects on impulsive excitation of ground surface coherent vibrational motion. A 'V' jump simulation

Allon Bartana; Uri Banin; Sanford Ruhman; Ronnie Kosloff

doi:10.1016/0009-2614(94)01055-2

Intensity effects on impulsive excitation of ground surface coherent vibrational motion. A 'V' jump simulation

Allon Bartana^*
, Uri Banin
, Sanford Ruhman
, Ronnie Kosloff

^*Corresponding author for this work

Institute of Chemistry

Research output: Contribution to journal › Article › peer-review

21 Scopus citations

Abstract

Control of coherent ground surface dynamics is achieved by varying the intensity of a resonant ultrafast pump pulse. This pulse cycles amplitude between the ground and excited electronic surfaces resulting in a momentum kick and a coordinate dependent loss of amplitude, creating a nonstationary vibrational distribution: the 'V' jump. A qualitative change in composition occurs for intensities above π pulse conditions. The induced dynamics is observed by a delayed pulse which is dispersed and analyzed against time or as a two-dimensional frequency plot. Such an analysis makes it possible to distinguish the contributions of high vibrational harmonics to the dynamics.

Original language	English
Pages (from-to)	211-217
Number of pages	7
Journal	Chemical Physics Letters
Volume	229
Issue number	3
DOIs	https://doi.org/10.1016/0009-2614(94)01055-2
State	Published - 28 Oct 1994

Bibliographical note

Funding Information:
This researchh asbeen supportedb y the Binational United States-Israel Science Foundation and the Israel Science foundation. The Farkas and the Fritz Haber Research Centers are supported by the Minerva Gesellschaft fur die Forschung, GmbH Munchen, FRG.

Access to Document

10.1016/0009-2614(94)01055-2

Cite this

@article{a5a3e431814443e69ddaf7e4d2dae32c,

title = "Intensity effects on impulsive excitation of ground surface coherent vibrational motion. A 'V' jump simulation",

abstract = "Control of coherent ground surface dynamics is achieved by varying the intensity of a resonant ultrafast pump pulse. This pulse cycles amplitude between the ground and excited electronic surfaces resulting in a momentum kick and a coordinate dependent loss of amplitude, creating a nonstationary vibrational distribution: the 'V' jump. A qualitative change in composition occurs for intensities above π pulse conditions. The induced dynamics is observed by a delayed pulse which is dispersed and analyzed against time or as a two-dimensional frequency plot. Such an analysis makes it possible to distinguish the contributions of high vibrational harmonics to the dynamics.",

author = "Allon Bartana and Uri Banin and Sanford Ruhman and Ronnie Kosloff",

note = "Funding Information: This researchh asbeen supportedb y the Binational United States-Israel Science Foundation and the Israel Science foundation. The Farkas and the Fritz Haber Research Centers are supported by the Minerva Gesellschaft fur die Forschung, GmbH Munchen, FRG.",

year = "1994",

month = oct,

day = "28",

doi = "10.1016/0009-2614(94)01055-2",

language = "אנגלית",

volume = "229",

pages = "211--217",

journal = "Chemical Physics Letters",

issn = "0009-2614",

publisher = "Elsevier B.V.",

number = "3",

}

TY - JOUR

T1 - Intensity effects on impulsive excitation of ground surface coherent vibrational motion. A 'V' jump simulation

AU - Bartana, Allon

AU - Banin, Uri

AU - Ruhman, Sanford

AU - Kosloff, Ronnie

N1 - Funding Information: This researchh asbeen supportedb y the Binational United States-Israel Science Foundation and the Israel Science foundation. The Farkas and the Fritz Haber Research Centers are supported by the Minerva Gesellschaft fur die Forschung, GmbH Munchen, FRG.

PY - 1994/10/28

Y1 - 1994/10/28

N2 - Control of coherent ground surface dynamics is achieved by varying the intensity of a resonant ultrafast pump pulse. This pulse cycles amplitude between the ground and excited electronic surfaces resulting in a momentum kick and a coordinate dependent loss of amplitude, creating a nonstationary vibrational distribution: the 'V' jump. A qualitative change in composition occurs for intensities above π pulse conditions. The induced dynamics is observed by a delayed pulse which is dispersed and analyzed against time or as a two-dimensional frequency plot. Such an analysis makes it possible to distinguish the contributions of high vibrational harmonics to the dynamics.

AB - Control of coherent ground surface dynamics is achieved by varying the intensity of a resonant ultrafast pump pulse. This pulse cycles amplitude between the ground and excited electronic surfaces resulting in a momentum kick and a coordinate dependent loss of amplitude, creating a nonstationary vibrational distribution: the 'V' jump. A qualitative change in composition occurs for intensities above π pulse conditions. The induced dynamics is observed by a delayed pulse which is dispersed and analyzed against time or as a two-dimensional frequency plot. Such an analysis makes it possible to distinguish the contributions of high vibrational harmonics to the dynamics.

UR - https://www.scopus.com/pages/publications/0001241894

U2 - 10.1016/0009-2614(94)01055-2

DO - 10.1016/0009-2614(94)01055-2

M3 - ???researchoutput.researchoutputtypes.contributiontojournal.article???

AN - SCOPUS:0001241894

SN - 0009-2614

VL - 229

SP - 211

EP - 217

JO - Chemical Physics Letters

JF - Chemical Physics Letters

IS - 3

ER -

Intensity effects on impulsive excitation of ground surface coherent vibrational motion. A 'V' jump simulation

Abstract

Bibliographical note

Access to Document

Other files and links

Fingerprint

Cite this