TY - JOUR
T1 - Large decrease in the critical temperature of superconducting LaFeAsO0.85 compounds doped with 3% atomic weight of nonmagnetic Zn impurities
AU - Guo, Y. F.
AU - Shi, Y. G.
AU - Yu, S.
AU - Belik, A. A.
AU - Matsushita, Y.
AU - Tanaka, M.
AU - Katsuya, Y.
AU - Kobayashi, K.
AU - Nowik, I.
AU - Felner, I.
AU - Awana, V. P.S.
AU - Yamaura, K.
AU - Takayama-Muromachi, E.
PY - 2010/8/5
Y1 - 2010/8/5
N2 - We observed a large decrease in Tc by no more than 3 at.% of Zn doped into the Tc -optimized superconductor LaFeAsO0.85 (Tc =26 K), confirmed by measurements of electrical resistivity, magnetic susceptibility, specific heat, Mössbauer spectroscopy, Hall coefficient, and an electron probe microanalysis. The rate ∼9 K/% is remarkably higher than others achieved by nonmagnetic impurities. The T c suppression is likely due to pair breaking caused by scattering associated with the highly localized electronic state of Zn in the Fe 2As2 layer. If this is true, the present result well accords with the theoretical prediction that suggests a sign reversal s -wave pairing model for the Fe-pnictide superconductors.
AB - We observed a large decrease in Tc by no more than 3 at.% of Zn doped into the Tc -optimized superconductor LaFeAsO0.85 (Tc =26 K), confirmed by measurements of electrical resistivity, magnetic susceptibility, specific heat, Mössbauer spectroscopy, Hall coefficient, and an electron probe microanalysis. The rate ∼9 K/% is remarkably higher than others achieved by nonmagnetic impurities. The T c suppression is likely due to pair breaking caused by scattering associated with the highly localized electronic state of Zn in the Fe 2As2 layer. If this is true, the present result well accords with the theoretical prediction that suggests a sign reversal s -wave pairing model for the Fe-pnictide superconductors.
UR - http://www.scopus.com/inward/record.url?scp=77957352044&partnerID=8YFLogxK
U2 - 10.1103/PhysRevB.82.054506
DO - 10.1103/PhysRevB.82.054506
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AN - SCOPUS:77957352044
SN - 1098-0121
VL - 82
JO - Physical Review B - Condensed Matter and Materials Physics
JF - Physical Review B - Condensed Matter and Materials Physics
IS - 5
M1 - 054506
ER -