TY - GEN
T1 - Observation of Raman-induced nuclear wavepacket motion in S1 cis-stilbene
T2 - Adiabatic change of a potential curvature and anharmonicity of multidimensional potential
AU - Takeuchi, Satoshi
AU - Ruhman, Sanford
AU - Ishii, Kunihiko
AU - Tahara, Tahei
PY - 2007
Y1 - 2007
N2 - Vibrational coherence was generated in S1 cis-stilbene at an optional delay time by the Raman process and the nuclear wavepacket motion was observed with 11-fs optical pulses. The frequency of the wavepacket motion exhibited gradual downshift with delaying timing of the creation, indicating highly anharmonic nature of the multi-dimensional S1 potential and a structural change proceeding in a picosecond time-scale.
AB - Vibrational coherence was generated in S1 cis-stilbene at an optional delay time by the Raman process and the nuclear wavepacket motion was observed with 11-fs optical pulses. The frequency of the wavepacket motion exhibited gradual downshift with delaying timing of the creation, indicating highly anharmonic nature of the multi-dimensional S1 potential and a structural change proceeding in a picosecond time-scale.
UR - http://www.scopus.com/inward/record.url?scp=62449312148&partnerID=8YFLogxK
U2 - 10.1007/978-3-540-68781-8_75
DO - 10.1007/978-3-540-68781-8_75
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AN - SCOPUS:62449312148
SN - 9783540687795
T3 - Springer Series in Chemical Physics
SP - 234
EP - 236
BT - Ultrafast Phenomena XV
PB - Springer New York
ER -