Observation of Raman-induced nuclear wavepacket motion in S1 cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential

Satoshi Takeuchi; Sanford Ruhman; Kunihiko Ishii; Tahei Tahara

doi:10.1007/978-3-540-68781-8_75

Observation of Raman-induced nuclear wavepacket motion in S₁ cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential

Satoshi Takeuchi^*
, Sanford Ruhman
, Kunihiko Ishii
, Tahei Tahara

^*Corresponding author for this work

Institute of Chemistry

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Abstract

Vibrational coherence was generated in S₁ cis-stilbene at an optional delay time by the Raman process and the nuclear wavepacket motion was observed with 11-fs optical pulses. The frequency of the wavepacket motion exhibited gradual downshift with delaying timing of the creation, indicating highly anharmonic nature of the multi-dimensional S₁ potential and a structural change proceeding in a picosecond time-scale.

Original language	English
Title of host publication	Ultrafast Phenomena XV
Subtitle of host publication	Proceedings of the 15th International Conference
Publisher	Springer New York
Pages	234-236
Number of pages	3
ISBN (Print)	9783540687795
DOIs	https://doi.org/10.1007/978-3-540-68781-8_75
State	Published - 2007

Publication series

Name	Springer Series in Chemical Physics
Volume	88
ISSN (Print)	0172-6218

Access to Document

10.1007/978-3-540-68781-8_75

Cite this

Takeuchi, S., Ruhman, S., Ishii, K., & Tahara, T. (2007). Observation of Raman-induced nuclear wavepacket motion in S₁ cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential. In Ultrafast Phenomena XV: Proceedings of the 15th International Conference (pp. 234-236). (Springer Series in Chemical Physics; Vol. 88). Springer New York. https://doi.org/10.1007/978-3-540-68781-8_75

Takeuchi, Satoshi ; Ruhman, Sanford ; Ishii, Kunihiko et al. / Observation of Raman-induced nuclear wavepacket motion in S₁ cis-stilbene : Adiabatic change of a potential curvature and anharmonicity of multidimensional potential. Ultrafast Phenomena XV: Proceedings of the 15th International Conference. Springer New York, 2007. pp. 234-236 (Springer Series in Chemical Physics).

@inproceedings{296ea36b4d8e490f9ce615ab1480040c,

title = "Observation of Raman-induced nuclear wavepacket motion in S1 cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential",

abstract = "Vibrational coherence was generated in S1 cis-stilbene at an optional delay time by the Raman process and the nuclear wavepacket motion was observed with 11-fs optical pulses. The frequency of the wavepacket motion exhibited gradual downshift with delaying timing of the creation, indicating highly anharmonic nature of the multi-dimensional S1 potential and a structural change proceeding in a picosecond time-scale.",

author = "Satoshi Takeuchi and Sanford Ruhman and Kunihiko Ishii and Tahei Tahara",

year = "2007",

doi = "10.1007/978-3-540-68781-8\_75",

language = "אנגלית",

isbn = "9783540687795",

series = "Springer Series in Chemical Physics",

publisher = "Springer New York",

pages = "234--236",

booktitle = "Ultrafast Phenomena XV",

address = "ארצות הברית",

}

Takeuchi, S, Ruhman, S, Ishii, K & Tahara, T 2007, Observation of Raman-induced nuclear wavepacket motion in S₁ cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential. in Ultrafast Phenomena XV: Proceedings of the 15th International Conference. Springer Series in Chemical Physics, vol. 88, Springer New York, pp. 234-236. https://doi.org/10.1007/978-3-540-68781-8_75

Observation of Raman-induced nuclear wavepacket motion in S₁ cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential. / Takeuchi, Satoshi; Ruhman, Sanford; Ishii, Kunihiko et al.
Ultrafast Phenomena XV: Proceedings of the 15th International Conference. Springer New York, 2007. p. 234-236 (Springer Series in Chemical Physics; Vol. 88).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

TY - GEN

T1 - Observation of Raman-induced nuclear wavepacket motion in S1 cis-stilbene

T2 - Adiabatic change of a potential curvature and anharmonicity of multidimensional potential

AU - Takeuchi, Satoshi

AU - Ruhman, Sanford

AU - Ishii, Kunihiko

AU - Tahara, Tahei

PY - 2007

Y1 - 2007

N2 - Vibrational coherence was generated in S1 cis-stilbene at an optional delay time by the Raman process and the nuclear wavepacket motion was observed with 11-fs optical pulses. The frequency of the wavepacket motion exhibited gradual downshift with delaying timing of the creation, indicating highly anharmonic nature of the multi-dimensional S1 potential and a structural change proceeding in a picosecond time-scale.

AB - Vibrational coherence was generated in S1 cis-stilbene at an optional delay time by the Raman process and the nuclear wavepacket motion was observed with 11-fs optical pulses. The frequency of the wavepacket motion exhibited gradual downshift with delaying timing of the creation, indicating highly anharmonic nature of the multi-dimensional S1 potential and a structural change proceeding in a picosecond time-scale.

UR - https://www.scopus.com/pages/publications/62449312148

U2 - 10.1007/978-3-540-68781-8_75

DO - 10.1007/978-3-540-68781-8_75

M3 - ???researchoutput.researchoutputtypes.contributiontobookanthology.conference???

AN - SCOPUS:62449312148

SN - 9783540687795

T3 - Springer Series in Chemical Physics

SP - 234

EP - 236

BT - Ultrafast Phenomena XV

PB - Springer New York

ER -

Takeuchi S, Ruhman S, Ishii K, Tahara T. Observation of Raman-induced nuclear wavepacket motion in S₁ cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential. In Ultrafast Phenomena XV: Proceedings of the 15th International Conference. Springer New York. 2007. p. 234-236. (Springer Series in Chemical Physics). doi: 10.1007/978-3-540-68781-8_75

Observation of Raman-induced nuclear wavepacket motion in S₁ cis-stilbene: Adiabatic change of a potential curvature and anharmonicity of multidimensional potential

Abstract

Publication series

Access to Document

Other files and links

Fingerprint

Cite this