Abstract
We relate the memory kernel in the Nakajima-Zwanzig-Mori time-convolution approach to the reduced system propagator which is often used to obtain the kernel in the Tokuyama-Mori time-convolutionless approach. The connection provides a robust and simple formalism to compute the memory kernel for a generalized system-bath model circumventing the need to compute high order system-bath observables, thus streamlining the use of numerically exact solvers for calculating the memory kernel. We illustrate this for a model system with electron-electron and electron-phonon couplings, driven away from equilibrium.
| Original language | English |
|---|---|
| Article number | 104105 |
| Journal | Journal of Chemical Physics |
| Volume | 149 |
| Issue number | 10 |
| DOIs | |
| State | Published - 14 Sep 2018 |
| Externally published | Yes |
Bibliographical note
Publisher Copyright:© 2018 Author(s).
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