Overcoming Frequency Resolution Limits Using a Solid-State Spin Quantum Sensor

The ability to determine precisely the separation of two frequencies is fundamental to spectroscopy, yet the resolution limit poses a critical challenge: distinguishing two incoherent signals becomes impossible when their frequencies are sufficiently close. Here, we demonstrate a simple and powerful approach, dubbed superresolution quantum sensing, which experimentally resolves two nearly identical incoherent signals using a solid-state spin quantum sensor. By carefully choosing interrogation times that satisfy the superresolution condition, we eliminate quantum projection noise, overcoming the vanishing distinguishability of signals with near-identical frequencies. This leads to improved resolution, which scales as t-2 in comparison to the standard t-1 scaling. Together with a greatly reduced classical readout noise assisted by a nuclear spin, we are able to achieve sub-kHz resolution with a signal detection time of 80 μs. Our results highlight the potential of quantum sensing to overcome conventional frequency resolution limitations, with broad implications for precision measurements.