Photodissociation of HBr adsorbed on the surface and embedded in large Arn clusters

Reinhard Baumfalk; Nils Hendrik Nahler; Udo Buck; Masha Y. Niv; R. Benny Gerber

doi:10.1063/1.481798

Photodissociation of HBr adsorbed on the surface and embedded in large Ar_n clusters

Reinhard Baumfalk, Nils Hendrik Nahler, Udo Buck, Masha Y. Niv, R. Benny Gerber

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Abstract

An experimental study was carried out focusing on the photodissociation dynamics of the two types of cluster geometries: the case where HBr is adsorbed at the surface of Ar_n and the case where the molecule is embedded within the rare-gas cluster. Calculations were carried out for different surface states of the larger system Ar₅₄(HCl) and Ar₅₅(HCl). The resulting data provide additional information on the cage effect for molecules at the surfaces in comparison with the cage effect in bulk.

Original language	English
Pages (from-to)	329-338
Number of pages	10
Journal	Journal of Chemical Physics
Volume	113
Issue number	1
DOIs	https://doi.org/10.1063/1.481798
State	Published - 1 Jul 2000

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Photodissociation of HBr adsorbed on the surface and embedded in large Ar_n clusters

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