Quantum Device Emulates the Dynamics of Two Coupled Oscillators

Ksenia Komarova, Hugo Gattuso, R. D. Levine, F. Remacle*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

19 Scopus citations

Abstract

Our quantum device is a solid-state array of semiconducting quantum dots that is addressed and read by 2D electronic spectroscopy. The experimental ultrafast dynamics of the device is well simulated by solving the time-dependent Schrödinger equation for a Hamiltonian that describes the lower electronically excited states of the dots and three laser pulses. The time evolution induced in the electronic states of the quantum device is used to emulate the quite different nonequilibrium vibrational dynamics of a linear triatomic molecule. We simulate the energy transfer between the two local oscillators and, in a more elaborate application, the expectation values of the quantum mechanical creation and annihilation operators of each local oscillator. The simulation uses the electronic coherences engineered in the device upon interaction with a specific sequence of ultrafast pulses. The algorithm uses the algebraic description of the dynamics of the physical problem and of the hardware.

Original languageEnglish
Pages (from-to)6990-6995
Number of pages6
JournalJournal of Physical Chemistry Letters
Volume11
Issue number17
DOIs
StatePublished - 3 Sep 2020

Bibliographical note

Publisher Copyright:
© 2020 American Chemical Society.

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