Quantum dynamics simulation of the ultrafast photoionization of Li2

Lorenzo Pesce; Zohar Amitay; Radoslaw Uberna; Stephen R. Leone; Mark Ratner; Ronnie Kosloff

doi:10.1063/1.1333004

Quantum dynamics simulation of the ultrafast photoionization of Li₂

Lorenzo Pesce, Zohar Amitay, Radoslaw Uberna, Stephen R. Leone, Mark Ratner, Ronnie Kosloff

Institute of Chemistry

Research output: Contribution to journal › Article › peer-review

35 Scopus citations

Abstract

The experimental pump/probe ultrafast photoionization of the lithium species were compared with the quantum dynamical calculations on potential energy surfaces. The perturbation techniques were used to analyze the quantum dynamics of signals obtained with different laser pulse shapes, intensities and chirps. The pumps show the inadequacies of the potential surfaces and dipole moment matrix elements of lithium dimer.

Original language	English
Pages (from-to)	1259-1271
Number of pages	13
Journal	Journal of Chemical Physics
Volume	114
Issue number	3
DOIs	https://doi.org/10.1063/1.1333004
State	Published - Jan 2001

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title = "Quantum dynamics simulation of the ultrafast photoionization of Li2",

abstract = "The experimental pump/probe ultrafast photoionization of the lithium species were compared with the quantum dynamical calculations on potential energy surfaces. The perturbation techniques were used to analyze the quantum dynamics of signals obtained with different laser pulse shapes, intensities and chirps. The pumps show the inadequacies of the potential surfaces and dipole moment matrix elements of lithium dimer.",

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Quantum dynamics simulation of the ultrafast photoionization of Li₂

Abstract

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