Abstract
We find an exact analytical solution to the exchange-only time-dependent density-functional theory (TDDFT) problem for a significant class of quasi-low-dimensional (QLD) materials: QLD electron gas with only one band filled in the direction perpendicular to the layer or wire. The theory yields the TD exchange potential as an explicit nonlocal operator of the TD spin density. The dressed interband (image states) excitation spectra of quasi-two-dimensional electron gas are obtained, while the comparison with the Kohn-Sham transitions provides insights into the qualitative and quantitative role of the many-body interactions. Important cancellations between the Hartree fH and the exchange fx kernels of TDDFT are found in the low-density regime, elucidating the interrelations between the Kohn-Sham and the many-body dynamics in mesoscopic systems.
| Original language | English |
|---|---|
| Article number | 236802 |
| Journal | Physical Review Letters |
| Volume | 118 |
| Issue number | 23 |
| DOIs | |
| State | Published - 8 Jun 2017 |
| Externally published | Yes |
Bibliographical note
Publisher Copyright:© 2017 American Physical Society.
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