Reduced parameter set determinable from geminate kinetics

Noam Agmon

doi:10.1016/j.cplett.2005.10.058

Reduced parameter set determinable from geminate kinetics

Noam Agmon^*

^*Corresponding author for this work

Institute of Chemistry

Research output: Contribution to journal › Article › peer-review

9 Scopus citations

Abstract

By fitting time-resolved measurements to models of diffusion influenced reactions it is possible to determine only parameters with no spatial dependence. The original set of distance-dependent parameters is reduced to a set of distance-independent parameters, and only these can be determined by fitting the model to the data. The present work demonstrates this point for reversible geminate recombination in one and three dimensions, showing how the reduced set of parameters is found by utilizing dimensional analysis or known analytic solutions. It is applied to the kinetic detection of proton-wires in the green fluorescent protein.

Original language	English
Pages (from-to)	530-534
Number of pages	5
Journal	Chemical Physics Letters
Volume	417
Issue number	4-6
DOIs	https://doi.org/10.1016/j.cplett.2005.10.058
State	Published - 10 Jan 2006

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10.1016/j.cplett.2005.10.058

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AB - By fitting time-resolved measurements to models of diffusion influenced reactions it is possible to determine only parameters with no spatial dependence. The original set of distance-dependent parameters is reduced to a set of distance-independent parameters, and only these can be determined by fitting the model to the data. The present work demonstrates this point for reversible geminate recombination in one and three dimensions, showing how the reduced set of parameters is found by utilizing dimensional analysis or known analytic solutions. It is applied to the kinetic detection of proton-wires in the green fluorescent protein.

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Reduced parameter set determinable from geminate kinetics

Abstract

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