Thermodynamics of mixed electrolyte solutions. XI. An isopiestic study of the quaternary system NaCl-KCl-CaCl2-H2O at 25°C

D. Saad*, J. Padova, Y. Marcus

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

4 Scopus citations

Abstract

Osmotic and activity coefficients in the aqueous quaternary system sodium chloride-potassium chloride-calcium chloride were derived from isopiestic measurements at 25°C. The isopiestic data were treated by the various procedures of Scatchard, Friedman, and Reilly, Wood, and Robinson. The results obtained showed good agreement with those obtained by pseudo-ternary transforms. Interaction parameters obtained indicated the preponderance of pairwise interactions. Excess Gibbs free energies of mixing were calculated.

Original languageEnglish
Pages (from-to)259-268
Number of pages10
JournalJournal of Solution Chemistry
Volume9
Issue number4
DOIs
StatePublished - Apr 1980

Keywords

  • Activity coefficients
  • excess Gibbs free energy of mixing
  • interaction parameters
  • NaCl:KCl:CaCl
  • osmotic coefficients

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