Three-body quenching of KrF* by Ar and broad-band emission at 415 nm

J. A. Mangano; J. H. Jacob; M. Rokni; A. Hawryluk

doi:10.1063/1.89465

Three-body quenching of KrF* by Ar and broad-band emission at 415 nm

J. A. Mangano^*
, J. H. Jacob
, M. Rokni
, A. Hawryluk

^*Corresponding author for this work

Research output: Contribution to journal › Article › peer-review

60 Scopus citations

Abstract

A kinetic model for the formation and quenching of KrF* ( ²Σ_1/2) that is applicable for electron-beam-excited mixtures of Ar/Kr/F₂ containing ≤15% Kr is presented. The product of the rate constant for the postulated three-body quenching process (KrF* +2 Ar→ArKrF*+Ar) and the KrF* lifetime is determined to be 5.2 ×10^-40 cm⁶. An exchange reaction (Kr+ArKrF*→Kr₂F*+Ar) rapidly leads to the formation of Kr₂F* whose emission is observed in a broad band centered at 415 nm. The KrF* laser saturation flux is given in terms of measured parameters and the mixture number density; for a 1-atm mixture with 0.3% F ₂ and 1% Kr it is 0.85 MW/cm².

Original language	English
Pages (from-to)	26-28
Number of pages	3
Journal	Applied Physics Letters
Volume	31
Issue number	1
DOIs	https://doi.org/10.1063/1.89465
State	Published - 1977
Externally published	Yes

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title = "Three-body quenching of KrF* by Ar and broad-band emission at 415 nm",

abstract = "A kinetic model for the formation and quenching of KrF* ( 2Σ1/2) that is applicable for electron-beam-excited mixtures of Ar/Kr/F2 containing ≤15\% Kr is presented. The product of the rate constant for the postulated three-body quenching process (KrF* +2 Ar→ArKrF*+Ar) and the KrF* lifetime is determined to be 5.2 ×10-40 cm6. An exchange reaction (Kr+ArKrF*→Kr2F*+Ar) rapidly leads to the formation of Kr2F* whose emission is observed in a broad band centered at 415 nm. The KrF* laser saturation flux is given in terms of measured parameters and the mixture number density; for a 1-atm mixture with 0.3\% F 2 and 1\% Kr it is 0.85 MW/cm2.",

author = "Mangano, \{J. A.\} and Jacob, \{J. H.\} and M. Rokni and A. Hawryluk",

year = "1977",

doi = "10.1063/1.89465",

language = "אנגלית",

volume = "31",

pages = "26--28",

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TY - JOUR

T1 - Three-body quenching of KrF* by Ar and broad-band emission at 415 nm

AU - Mangano, J. A.

AU - Jacob, J. H.

AU - Rokni, M.

AU - Hawryluk, A.

PY - 1977

Y1 - 1977

N2 - A kinetic model for the formation and quenching of KrF* ( 2Σ1/2) that is applicable for electron-beam-excited mixtures of Ar/Kr/F2 containing ≤15% Kr is presented. The product of the rate constant for the postulated three-body quenching process (KrF* +2 Ar→ArKrF*+Ar) and the KrF* lifetime is determined to be 5.2 ×10-40 cm6. An exchange reaction (Kr+ArKrF*→Kr2F*+Ar) rapidly leads to the formation of Kr2F* whose emission is observed in a broad band centered at 415 nm. The KrF* laser saturation flux is given in terms of measured parameters and the mixture number density; for a 1-atm mixture with 0.3% F 2 and 1% Kr it is 0.85 MW/cm2.

AB - A kinetic model for the formation and quenching of KrF* ( 2Σ1/2) that is applicable for electron-beam-excited mixtures of Ar/Kr/F2 containing ≤15% Kr is presented. The product of the rate constant for the postulated three-body quenching process (KrF* +2 Ar→ArKrF*+Ar) and the KrF* lifetime is determined to be 5.2 ×10-40 cm6. An exchange reaction (Kr+ArKrF*→Kr2F*+Ar) rapidly leads to the formation of Kr2F* whose emission is observed in a broad band centered at 415 nm. The KrF* laser saturation flux is given in terms of measured parameters and the mixture number density; for a 1-atm mixture with 0.3% F 2 and 1% Kr it is 0.85 MW/cm2.

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JO - Applied Physics Letters

JF - Applied Physics Letters

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Three-body quenching of KrF* by Ar and broad-band emission at 415 nm

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