Three-dimensional simulations of reversible bimolecular reactions. II. The excited-state target problem with different lifetimes

Alexander V. Popov; Noam Agmon

doi:10.1063/1.1496455

Three-dimensional simulations of reversible bimolecular reactions. II. The excited-state target problem with different lifetimes

Alexander V. Popov, Noam Agmon^*

^*Corresponding author for this work

Institute of Chemistry

Research output: Contribution to journal › Article › peer-review

21 Scopus citations

Abstract

Three-dimensional simulations of reversible bimolecular reaction in 3D with different excited state lifetimes were reported. Quantitative comparison between various theories and simulation was presented. Pre-equilibrium approximation was obtained, when the excited species equilibrate fast compared with the excited-state lifetimes. The quasistationary approximation was observed during the fast excited-state decay of the particles.

Original language	English
Pages (from-to)	4376-4385
Number of pages	10
Journal	Journal of Chemical Physics
Volume	117
Issue number	9
DOIs	https://doi.org/10.1063/1.1496455
State	Published - 1 Sep 2002

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abstract = "Three-dimensional simulations of reversible bimolecular reaction in 3D with different excited state lifetimes were reported. Quantitative comparison between various theories and simulation was presented. Pre-equilibrium approximation was obtained, when the excited species equilibrate fast compared with the excited-state lifetimes. The quasistationary approximation was observed during the fast excited-state decay of the particles.",

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AB - Three-dimensional simulations of reversible bimolecular reaction in 3D with different excited state lifetimes were reported. Quantitative comparison between various theories and simulation was presented. Pre-equilibrium approximation was obtained, when the excited species equilibrate fast compared with the excited-state lifetimes. The quasistationary approximation was observed during the fast excited-state decay of the particles.

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Three-dimensional simulations of reversible bimolecular reactions. II. The excited-state target problem with different lifetimes

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