Time-resolved dissociative ionization and double photoionization of CO2

Dror M. Bittner, Krishnendu Gope, Daniel Strasser*

*Corresponding author for this work

Research output: Contribution to journalArticlepeer-review

10 Scopus citations

Abstract

CO2 single-photon double photoionization, Coulomb explosion, and dissociative ionization are studied with ultrafast extreme-ultraviolet pump and time-delayed near-infrared probe pulses. Kinetic energy release and momentum correlations for the two-body CO+ + O+ and three-body O+ + C+ + O fragmentation products are determined by 3D coincidence fragment imaging. The transient enhancement of the ratio of two-body vs three-body Coulomb explosion events and the time dependence of low and high kinetic energy release dissociation events are discussed in terms of dissociative ionization and Coulomb explosion dynamics.

Original languageAmerican English
Article number194201
JournalJournal of Chemical Physics
Volume153
Issue number19
DOIs
StatePublished - 21 Nov 2020

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