Abstract
The Tannor-Rice pump-dump scheme for controlling the selectivity of product formation in a chemical reaction is improved by development of a method for optimizing the field of a particular product with respect to the shapes of the pump and dump pulses. Numerical studies of the optimization of product yield in a model system of the same type as studied by Tannor and Rice illustrate the enhancement possible with pulse shaping.
Original language | English |
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Pages (from-to) | 201-220 |
Number of pages | 20 |
Journal | Chemical Physics |
Volume | 139 |
Issue number | 1 |
DOIs | |
State | Published - 1 Dec 1989 |