Wavepacket dancing: Achieving chemical selectivity by shaping light pulses

R. Kosloff; S. A. Rice; P. Gaspard; S. Tersigni; D. J. Tannor

doi:10.1016/0301-0104(89)90012-8

Wavepacket dancing: Achieving chemical selectivity by shaping light pulses

R. Kosloff^*, S. A. Rice, P. Gaspard, S. Tersigni, D. J. Tannor

^*Corresponding author for this work

Institute of Chemistry

Research output: Contribution to journal › Article › peer-review

719 Scopus citations

Abstract

The Tannor-Rice pump-dump scheme for controlling the selectivity of product formation in a chemical reaction is improved by development of a method for optimizing the field of a particular product with respect to the shapes of the pump and dump pulses. Numerical studies of the optimization of product yield in a model system of the same type as studied by Tannor and Rice illustrate the enhancement possible with pulse shaping.

Original language	English
Pages (from-to)	201-220
Number of pages	20
Journal	Chemical Physics
Volume	139
Issue number	1
DOIs	https://doi.org/10.1016/0301-0104(89)90012-8
State	Published - 1 Dec 1989

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10.1016/0301-0104(89)90012-8

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Wavepacket dancing: Achieving chemical selectivity by shaping light pulses

Abstract

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